![]() The effect of interfacial deformation on electrodeposition kinetics. Lithium mechanics: roles of strain rate and temperature and implications for lithium metal batteries. Review-practical challenges hindering the development of solid state Li ion batteries. ![]() Kerman, K., Luntz, A., Viswanathan, V., Chiang, Y.-M. An in vivo formed solid electrolyte surface layer enables stable plating of Li metal. Relevance of solid electrolytes for lithium-based batteries: a realistic view. Mechanism of lithium metal penetration through inorganic solid electrolytes. Suppressing Li dendrite formation in Li 2S-P 2S 5 solid electrolyte by LiI incorporation. Elastic, plastic, and creep mechanical properties of lithium metal. Masias, A., Felten, N., Garcia-Mendez, R., Wolfenstine, J. Continuous plating/stripping behavior of solid-state lithium metal anode in a 3D ion-conductive framework. Interface-engineered all-solid-state Li-ion batteries based on garnet-type fast Li+ conductors. Li metal deposition and stripping in a solid-state battery via Coble creep. Mechanical properties of metallic lithium: from nano to bulk scales. ![]() Fundamentals of inorganic solid-state electrolytes for batteries. Recent advances in rechargeable battery materials: a chemist’s perspective. Challenges and perspectives for new material solutions in batteries. Pellegrini, V., Bodoardo, S., Brandell, D. As a result, cracks traverse the entire electrolyte before the Li arrives at the other electrode, and therefore before a short circuit occurs. ![]() Lithium ingress drives the propagation of the spallation and transverse cracks by widening the crack from the rear that is, the crack front propagates ahead of the Li. Transverse cracks then propagate from the spallations across the electrolyte from the plated to the stripped electrode. The spallations form predominantly at the lithium electrode edges where local fields are high. On plating, cracking initiates with spallation, conical ‘pothole’-like cracks that form in the ceramic electrolyte near the surface with the plated electrode. Utilizing in situ X-ray computed tomography coupled with spatially mapped X-ray diffraction, the propagation of cracks and the propagation of lithium dendrites through the solid electrolyte have been tracked in a Li/Li 6PS 5Cl/Li cell as a function of the charge passed. Lithium dendrite (filament) propagation through ceramic electrolytes, leading to short circuits at high rates of charge, is one of the greatest barriers to realizing high-energy-density all-solid-state lithium-anode batteries. ![]()
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